Carbon-based materials, especially graphene, have the advantages of broadband absorption and excellent photothermal properties, and hold promise for solar–thermal energy conversion. However, to date, graphene-based solar–thermal materials with superior omnidirectional light harvesting performances remain elusive.
Previously, a 90-nm-thick graphene grating metamaterial with ~85% absorptivity of unpolarized light covering almost the entire solar spectrum was demonstrated 29. However, the ultrabroadband absorption is incapable of designing a selective solar absorber due to the challenge in limiting the absorption in the desired cut-off wavelength range.
The large effective area of the graphene metamaterial sidewalls within the high electric field intensity regime leads to most of the light being absorbed by the ultrathin graphene metamaterial layer, as displayed in Fig. 2b, and subsequently be converted to thermal energy.
Therefore, the photo-generated heat in the graphene metamaterial layer on SGM absorber can be readily conducted through this continuous metamaterial film for further usage since the graphene metamaterials feature excellent thermal conductivity, while hardly dispersed by thermal radiation.
Scalable and low-cost synthesis of black amorphous Al-Ti-O nanostructure for high-efficient photothermal desalination Synthetic graphene oxide leaf for solar desalination with zero liquid discharge Environ. Sci.
Herein, we demonstrate that by conformally coating a 30-nm-thick graphene metamaterial on a 3D trench-like structure to form the SGM, the exact absorption band for efficient solar-selective absorption can be precisely controlled.
Scalable Production of Integrated Graphene Nanoarchitectures for ...
Here we report a hierar-chical nanoarchitecture that integrates vertically oriented graphene nanosheets and highly porous graphene aerogel to achieve ultrafast solar-thermal response (a …
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Efficient and scalable solar energy harvesting for thermoelectric ...
Furtherly, the resultant photothermal graphene promoted thermoelectric generator has been obtained and shows an outstanding combination of strong solar irradiation absorption (more than 97%), excellent photothermal conversion ability, and extraordinary anti-fouling performance (a large water contact angle of more than 150° and small ...
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Functionalized Graphene Enables Highly Efficient Solar Thermal …
Here, we demonstrate that functionalizing graphene using hydrophilic groups can greatly enhance the solar thermal steam generation efficiency. Our results show that specially functionalized graphene can improve the overall solar-to-vapor efficiency from 38% to 48% at one sun conditions compared to chemically reduced graphene oxide. Our ...
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Sustainable Production of Graphene from Solar‐Driven Expanded …
2 · The electromagnetic interference (EMI) shielding properties of solar graphene are evaluated in the X-band region, ... However, the energy consumption in the existing thermal and microwave-assisted expansion processes is very high, around 500 and 63 MJ. [44, 46] To achieve graphene sheets with a large lateral size and minimal energy consumption through the liquid …
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Hybrid photothermal structure based on Cr-MgF2 solar …
Hybrid photothermal structure that can efficiently manage solar heat is suggested. It consists of a Cr/MgF 2 multi-layered film and a PMMA-graphene heat reservoir layer. Hybrid photothermal structure shows high light absorption over 90% in visible light wavelengths.
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Graphene quantum dots as game-changers in solar cell ...
Graphene quantum dots (GQDs) are zero-dimensional carbonous materials with exceptional physical and chemical properties such as a tuneable band gap, good conductivity, quantum confinement, and edge effect. The introduction of GQDs in various layers of solar cells (SCs) such as hole transport layer (HTL), electron transport materials (ETM), …
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Graphene-based thermionic-thermoradiative solar cells: Concept ...
Solar energy conversion to electricity usually adopts two main methods: photovoltaic and solar-thermal power generation. Here, graphene-based thermionic-thermoradiative solar cells are expanded to include photovoltaics based on thermionic-thermoradiative converters, hybrid concept, efficiency limit, and optimum design.
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Structured graphene metamaterial selective absorbers for high ...
An ideal solar-thermal absorber requires efficient selective absorption with a tunable bandwidth, excellent thermal conductivity and stability, and a simple structure for effective solar...
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Functionalized Graphene Enables Highly Efficient Solar Thermal …
KEYWORDS: functionalized graphene, hydrophilic groups, solar steam generation, high efficiency evaporation, vapor−liquid interface S olar irradiation is the most abundant renewable energy
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Hybrid photothermal structure based on Cr-MgF2 solar …
Hybrid photothermal structure that can efficiently manage solar heat is suggested. It consists of a Cr/MgF 2 multi-layered film and a PMMA-graphene heat reservoir layer. Hybrid …
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Graphene-based thermionic-thermoradiative solar cells: Concept ...
Solar energy conversion to electricity usually adopts two main methods: photovoltaic and solar-thermal power generation. Here, graphene-based thermionic-thermoradiative solar cells are expanded to include photovoltaics based on thermionic-thermoradiative converters, hybrid concept, efficiency limit, and optimum design. For realistic …
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Hierarchical Graphene Foam for Efficient Omnidirectional Solar–Thermal …
Herein, hierarchical graphene foam (h-G foam) with continuous porosity grown via plasma-enhanced chemical vapor deposition is reported, showing dramatic enhancement of broadband and omnidirectional absorption of sunlight, which thereby can enable a considerable elevation of temperature.
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Hygroscopic assisted solar photo-thermal-electric conversion …
However, the solar efficiency of this work is not ideal, which is less than 30 % [41], [42], [43]. Therefore, it is very necessary to design an advanced photo-thermal-electric system with long-term power generation at night and …
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Progress in 3D-Graphene Assemblies Preparation for Solar …
This review is a valuable reference for the development of 3D-graphene materials and solar-thermal steam generation and water treatment. Key words: Graphene, Three-dimensional …
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Solar Thermoelectricity for Power Generation
Solar optical concentrators, thermal and selective absorbers, and other tools are proposed to improve the performance of solar thermoelectrics. Despite continuous research and development, experimental solar thermoelectric efficiencies remain below 10%, and theoretical efficiencies do not surpass 20%. In this review, the different designs of solar thermoelectric generators are …
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Progress in 3D-Graphene Assemblies Preparation for Solar-Thermal …
This review is a valuable reference for the development of 3D-graphene materials and solar-thermal steam generation and water treatment. Key words: Graphene, Three-dimensional structure,...
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Scalable Production of Integrated Graphene Nanoarchitectures for ...
Here we report a hierarchical nanoarchitecture that integrates vertically oriented graphene nanosheets and highly porous graphene aerogel to achieve ultrafast solar-thermal …
Learn More
Functionalized Graphene Enables Highly Efficient …
Here, we demonstrate that functionalizing graphene using hydrophilic groups can greatly enhance the solar thermal steam generation efficiency. Our results show that specially functionalized ...
Learn More
Scalable Production of Integrated Graphene Nanoarchitectures …
Here we report a hierar-chical nanoarchitecture that integrates vertically oriented graphene nanosheets and highly porous graphene aerogel to achieve ultrafast solar-thermal response (a temperature increase of 169.7 C within 1 s), resulting from superior photonic absorption and excellent thermal insulation.
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Scalable Production of Integrated Graphene Nanoarchitectures for ...
Here we report a hierarchical nanoarchitecture that integrates vertically oriented graphene nanosheets and highly porous graphene aerogel to achieve ultrafast solar-thermal response (a temperature increase of 169.7°C within 1 s), resulting from superior photonic absorption and excellent thermal insulation.
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Hierarchical Graphene Foam for Efficient …
Herein, hierarchical graphene foam (h-G foam) with continuous porosity grown via plasma-enhanced chemical vapor deposition is reported, showing dramatic enhancement of broadband and omnidirectional absorption …
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Enhanced interfacial solar steam generation with composite …
To improve the efficiency of solar steam generation, many work focused on improving solar light absorption and reducing thermal losses. Recently, nanometer-sized particles (NPs) (Cho et al., 2015), have gained much attention as a photo-thermal conversion medium.Nanofluid is a type of fluid suspension containing NPs (Amjad et al., 2017, Eastman …
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Scalable Production of Integrated Graphene Nanoarchitectures …
Solar energy harvesting, particularly solar-thermal conversion, has received recent attention for applications such as DNA sequencing, medical sterilization, power generation, de-icing, tumor cell ablation, and seawater desalination. 1–6 Among these techniques, solar-thermal vapor generation has become one of the most attractive green and renewable …
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Graphene-based thermionic-thermoradiative solar cells: Concept ...
Solar energy conversion to electricity usually adopts two main methods: photovoltaic and solar-thermal power generation. Here, graphene-based thermionic …
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Functionalized Graphene Enables Highly Efficient Solar …
Here, we demonstrate that functionalizing graphene using hydrophilic groups can greatly enhance the solar thermal steam generation efficiency. Our results show that specially functionalized graphene can improve the overall solar-to-vapor …
Learn More
Sustainable Production of Graphene from Solar‐Driven Expanded …
2 · The electromagnetic interference (EMI) shielding properties of solar graphene are evaluated in the X-band region, ... However, the energy consumption in the existing thermal …
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Hybrid photothermal structure based on Cr-MgF2 solar …
Hybrid photothermal structure based on Cr-MgF 2 solar absorber/PMMA-graphene heat reservoir for enhanced thermoelectric power generation. Author links open overlay panel Geonho Kwak a, Yoo-Seok Jeong b, Sun-Woo Kim b, Jin-Kyeom Kim b, Jihyeok Choi c, Kyung Guen Song c d, Hee Jun Kim e, Won Jun Choi e, Ya Yang f, Hyun-Cheol Song b g h, …
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Efficient and scalable solar energy harvesting for thermoelectric ...
Furtherly, the resultant photothermal graphene promoted thermoelectric generator has been obtained and shows an outstanding combination of strong solar irradiation …
Learn More
Structured graphene metamaterial selective absorbers for high ...
An ideal solar-thermal absorber requires efficient selective absorption with a tunable bandwidth, excellent thermal conductivity and stability, and a simple structure for …
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Sequential Bayesian-optimized graphene synthesis by direct solar ...
(a) Overview of solar-thermal CVD setup for graphene synthesis. (b) Flow chart for graphene synthesis parameters.(c) Copper substrate temperature profile prior to graphene growth computed by a ...
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