A large number of studies show that the charge-discharge ratio of aging battery is significantly higher than that of normal capacity battery. When the charge-discharge current and cut-off voltage exceed a certain threshold, the capacity attenuation accelerates.
The aging mode of the battery is quantified by the capacity ratio of electrodes and the SOC bias of the positive electrode. To better understand the variation of internal parameters with battery aging, the simplified electrochemical model is used to identify the parameters in Ref. [ 24 ].
To identify the aging mechanism of the battery by using the OCV curve of electrodes, it is necessary to establish the correlation model between the aging and the OCV curves. Besides, considering that the SOC i of the electrode can not be measured directly, it is necessary to map the SOC of the whole battery to the electrode SOC i.
The charging and discharging capacity of batteries with high aging degree will change significantly under extreme conditions [83, 84]. However, the capacity attenuation of the battery during aging can be expressed by SOH, and the estimated correction of SOC must also depend on the SOH .
The attenuation of electrical power is mainly due to the change of the equivalent resistance of the battery, which is also caused by side reactions and the rupture of the electrode structure, And the common manifestation is the generation of a solid electrolyte interface (SEI) film on the electrode surface.
In this work, the aging factors of lithium batteries are classified, and the influence of positive and negative aging of battery on lithium battery is analyzed. The aging mechanism of lithium battery is divided into the loss of active lithium ion (LLI), the loss of active material (LAM) and the increase of internal resistance.
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