The first groundbreaking solar battery concept of combined solar energy harvesting and storage was investigated in 1976 by Hodes, Manassen, and Cahen, consisting of a Cd–Se polycrystalline chalcogenide photoanode, capable of light absorption and photogenerated electron transfer to the S 2– /S redox couple in the electrolyte.
Since no external wires are required for photocharging and a BAM is employed, this solar battery design represents a very high level of integration. By performing both light absorption and charge storage, bifunctional materials enable the most recent and highest level of material integration in solar batteries.
By performing both light absorption and charge storage, bifunctional materials enable the most recent and highest level of material integration in solar batteries. To conclude, bifunctional materials are the most recent development in solar battery research.
In summary, bifunctional electrodes present the next step of integrated solar battery designs. Only two electrodes are required, since one of the electrodes is capable of effectively performing two functions: light absorption and charge storage.
A similar device has recently also been published for Li–S batteries. (40) To conclude, the family of devices consisting of three electrodes in one enclosure presents a further step toward integration and marks a significant milestone in the solar battery field.
Solar batteries present an emerging class of devices which enable simultaneous energy conversion and energy storage in one single device. This high level of integration enables new energy storage concepts ranging from short-term solar energy buffers to light-enhanced batteries, thus opening up exciting vistas for decentralized energy storage.
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